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Beilstein J. Org. Chem. 2019, 15, 2473–2485, doi:10.3762/bjoc.15.240
Graphical Abstract
Scheme 1: PSHD photochromism [10].
Figure 1: Proposed gating of sensitivity to photoinduced charge transfer by a photochromic photooxidant in wh...
Scheme 2: QSHD photochromism [21].
Figure 2: Cyclic voltammograms of a) 1b before irradiation or electrolysis (solid blue), b) 1b/2b after 25 sc...
Figure 3: Cyclic voltammograms of a) 3b (with trace 5b) before irradiation or electrolysis (solid blue), b) 3b...
Figure 4: Cyclic voltammograms of a) 3a before irradiation or electrolysis (solid blue), b) 3a + 5a after 25 ...
Figure 5: 1H NMR distinction between SW 3a, thermal/eLW 5a, and pLW 4a, in acetone-d6, as observed a) before ...
Figure 6: HOMO (MO 105, red and blue) and LUMO (MO 106, green and yellow) computed for 3a in its ground (S0) ...
Scheme 3: Proposed mechanism for differential formation of pLW (4) and eLW (5) from SW (3).
Figure 7: Frontier orbital occupancies of relevant electronic states of 3a. Note: the photochemical excited s...